if you just want to do it for your iTunes just right click on the song and then click get info, then go to album artwork and copy and paste your picture in (to do it for multiple items hold shift and click on the last song you want to change the picture for)
A much faster way to do this is in Windows Media player. You should import the music and then right click on the song or album and select get album art. You then just pick the one you want of the data bank. If this doesn't work you can copy and paste the album art where it's meant to go.
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