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These made great Christmas ornaments on our small tree!I used 20 gauge brightly colored enameled copper wire.I'd suggest not using anything heavier than 18 gauge wire - mainly because that's pretty hard on your hands even if you have really good tools. Anything finer than 22 gauge won't be durable enough for every day wear unless your pendants are really small (24 gauge for earrings, perhaps!)A note of caution - working hard wire (like memory wire) will really tear up your wrists over time, if you're doing intricate bends like this. Look for soft wire instead.
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