I've tried to mod my controller and it's pretty hard, although I'm not an expert at mods, but I've taken my 360 controllers apart many times. I took out the piece that directs the lights so you can see it through at most of the controller, butwhen I put it together, L1 and R1 didn't work, so I tried taking it apart again and ALL the shoulder buttons didn't work! So it's still in pieces in my basement. : \
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u can get a custom ps3 controller skin I've seen a vid of a guy who connected it to a rc hellicopter on you tube
chopping it in half with a bandsaw would be a 'mod'.
What do you want to change?
The LEDs can be changed for colours, or moved around. Dualshock can be ...shockier. You could put a bigger equivelant battery in.
The pressure sensitive buttons with goofy matrixing make it RIDICULOUSLY difficult to add rapid fire, etc.