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Absolutely, although I recommend using a filler material once you start looking into bigger pieces. The thicker it is the longer it takes to dry and the heavier it is. You'll also use up more material and have to make more.I've used it solid for teeth/claws/bone as big as my pinky - so a little more than .75 inch at the thickest and about 3 inches long and it dried up quickly and firmly enough. You're probably good at twice that size but at that point it starts to make sense to use filler material like expanding foam to build your base and then cover it with a few layers of paper clay especially if you're looking at using this for costuming.
Animator Gadget for NeoPixels
Bubbling Pipe Lamp
Laser Cut Jewelry: Layered Acrylic Rings
High Volume Rain Barrel
Alien Mercenary Halloween Costume
Hydraulic Ram Pump
T-Rex Dinosaur Puzzle with different sizes and positions
Maze Ball Mask (laser cut)
How to make a Scary Scarecrow Mask (With Moveable Jaw)
How to Build a 12x20 Cabin on a Budget
How to Make a Paper Hat
Mini tophat fascinator
Wickie Helmet (Vicke Viking)
Easy & Adorable Owl Costume
Loud foghorn from plumbing parts
Arcade Button MIDI Controller
Simple Animatronics (robotic hand)
How to Build an Earthbag Roundhouse
Shake it like a Tic-Tac!
How I built an electricity producing wind turbine
Touch Sensitive RGB LED Mood Light
Permanently Changing The Background In Windows 7 Starter
How To Make Your Own Sugru Substitute
Supercapacitor USB Light
Mini Altoid Gas Grill
Flashlight with no batteries
Chainsaw flashlight (gas engine powered spotlight)
Kentucky Fried WTF on a stick
Sand Fire Garden
Blinking Nightlight (by request)
USB Iphone Ipod Dynamo Charger
Dried Fruit Rolls
Spooky Tesla Spirit Radio
Audio Cassette Loop
Bright Luxeon LED Bike Light
RGB Color Controllable High Power LED Room + Spot Lighting
String Pendant Lamp
Another Benchtop Power Supply from PC Power Supply
Super simple high power LED driver
Friendly Folding Keychain
Weekly Project: Voltoids; or, How to Make 5V from 1.5V
Rain or Shine Solar Charger
Make an amazing sports noisemaker!
Bison Horns and Ears on an Elastic Headband
How to build a Sami hut in wood!
How to make sci-fi / steampunk goggles from trash.
Baby Dragon Cape
Distortion For Cheap!
Modular "Flunk" Synth
Making Music with an Atari Punk Console
Build a D-Ring Bit driver
Test Tools: A fairly simple 555 tester. Corrected and updated.
Simple overdrive effect pedal
No More Roaches
Rubber Hose Chair
Tic Tac Tunes - Now with Tic Tac Beat Box
Building a drum machine with low-cost tangible interface (d-touch drum machine)
A wearable sound-to-light display, without a microprocessor - the Musicator Junior.
Simple music light show (lpt led)
Birth of Man Mixing Board
The Minty Kalimba
Listen to a led tea light
A More Annoying Noise Maker (Version 1.0)
Nandhopper 1-Bit Noise Synth
Make A Handheld Solar Power Supply
D.I.Y. Screen Printing